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論文

Estimation for mass transfer coefficient under two-phase flow conditions using two gas components

南上 光太郎; 塩津 弘之; 丸山 結; 杉山 智之; 岡本 孝司*

Journal of Nuclear Science and Technology, 60(7), p.816 - 823, 2023/07

 被引用回数:0 パーセンタイル:0.01(Nuclear Science & Technology)

For proper source term evaluation, we constructed the theoretical model to estimate the mass transfer coefficient of gaseous iodine species under two-phase flow conditions, which complicates the direct experimental measurements. The mass transfer speed is determined by the product of the overall mass transfer coefficient and the interfacial area. By using the ratio of two gas components, the interfacial area, which is an important parameter that is difficult to measure, can be canceled out and the ratio of their overall mass transfer coefficients can be obtained. This ratio is expected to be equal to the ratio of their diffusion coefficients. Therefore, the unknown mass transfer coefficient such as iodine species can be estimated using the diffusion coefficients of two gas components and the reference mass transfer coefficient such as O$$_{2}$$. We carried out the experiments using the bubble column to confirm this relationship. From the results in this study, we confirmed that the ratio of the overall mass transfer coefficient was in good agreement with the ratio of diffusion coefficient under the bubbly flow conditions. Using this relationship confirmed in this study, we estimated the mass transfer coefficient of I$$_{2}$$, one of the iodine species.

論文

Revolatilization of iodine by bubbly flow in the suppression pool during an accident

南上 光太郎; 石川 淳; 杉山 智之; Pellegrini, M.*; 岡本 孝司*

Journal of Nuclear Science and Technology, 59(11), p.1407 - 1416, 2022/11

 被引用回数:7 パーセンタイル:90.45(Nuclear Science & Technology)

To appropriately evaluate the amount of radioactive iodine released into the environment, we extended the current pool scrubbing model to consider revolatilization at bubble surfaces due to bubbly flow generated in the suppression pool, and the effect of revolatilization by bubbly flow was quantitatively evaluated using a station black out sequence in this work. Gaseous iodine species are produced in the suppression pool in an accident. They are gradually released from the pool surface, but when a large amount of gas flows from the drywell into the suppression pool, the revolatilization of gaseous iodine dissolved in the pool water is promoted by bubbly flow. The results of this study indicated that the release amount of iodine immediately after suppression chamber (S/C) vent operation increased by up to 134 times when considering the revolatilization effect associated with bubbly flow. These results were due to the increase in the gas-liquid interfacial area at bubble surfaces and the overall mass transfer coefficients under two-phase flow conditions due to bubbly flow. It was shown that caution is required for early S/C vent operation.

論文

A Comparative CFD exercise on bubble hydrodynamics using Euler-Euler and interface tracking approaches

Dehbi, A.*; Cheng, X.*; Liao, Y.*; 岡垣 百合亜; Pellegrini, M.*

Proceedings of 19th International Topical Meeting on Nuclear Reactor Thermal Hydraulics (NURETH-19) (Internet), 15 Pages, 2022/03

Nuclear degraded cores produce fission product aerosols that may reach the environment if not removed by natural processes and/or filtering equipment. The transport paths of aerosols usually include transits through stagnant water pools. It is therefore essential to develop computational tools to predict the aerosols retention by water pools. Currently, this is mostly done with 1-D lumped-parameter codes that are too simplistic to capture the physics. It is hence worthwhile to attempt the CFD approach, which has recently become reasonably mature to address bubble hydrodynamics in low momentum two-phase flows. In this first comparative exercise, we restrict the investigation to a hypothetical parallelepiped water pool (2$$times$$2$$times$$8 cm$$^{3}$$) into which air is injected through a circular 4 mm ID orifice at low velocity of 0.2 m/s. We present predictions of the gas phase dynamics (void and velocity profiles) for both Euler-Euler and Interface Tracking (IT, Volume-of-Fluid (VOF)) methodologies. In addition, we compare bubble shape, volume and detachment frequency from various IT simulation codes (CFX, Fluent, Star-CCM+, OpenFOAM). Reasonable agreement is found between IT simulations near the injector, but discrepancies increase as one moves towards the free surface. The disagreement between the Euler-Euler and IT results is substantial throughout the domain. Future studies will consist of validation exercises against experimental data to highlight potential model deficiencies and point to ways of remedying them.

論文

Integration of pool scrubbing research to enhance source-term calculations (IPRESCA) project

Gupta, S.*; Herranz, L. E.*; Lebel, L. S.*; Sonnenkalb, M.*; Pellegrini, M.*; Marchetto, C.*; 丸山 結; Dehbi, A.*; Suckow, D.*; K$"a$rkel$"a$, T.*

Proceedings of 19th International Topical Meeting on Nuclear Reactor Thermal Hydraulics (NURETH-19) (Internet), 16 Pages, 2022/03

Pool scrubbing is a major topic in water cooled nuclear reactor technology as it is one of the means for mitigating the source-term to the environment during a severe accident. Pool scrubbing phenomena include coupled interactions between bubble hydrodynamics, aerosols and gaseous radionuclides retention mechanisms under a broad range of thermal-hydraulic conditions as per accident scenarios. Modeling pool scrubbing in some relevant accident scenarios has shown to be affected by substantial uncertainties. In this context, IPRESCA (Integration of Pool scrubbing Research to Enhance Source-term CAlculations) project aims to promote a better integration of international research activities related to pool scrubbing by providing support in experimental research to broaden the current knowledge and database, and by supporting analytical research to facilitate systematic validation and model enhancement of the existing pool scrubbing codes. The project consortium includes more than 30 organisations from 15 countries involving research institutes, universities, TSOs, and industry. For IPRESCA activities, partners join the project with in-kind contributions. IPRESCA operates under NUGENIA Technical Area 2/SARNET (Severe Accident) - Sub Technical Area 2.4 (Source-term). The present paper provides an introduction and overview of the IPRESCA project, including its objectives, organizational structure and the main outcomes of completed activities. Furthermore, key activities currently ongoing or planned in the project framework are also discussed.

口頭

Radionuclides release behaviors unique to the Fukushima Daiichi Nuclear Power Plants accident

日高 昭秀

no journal, , 

During the Fukushima Daiichi NPP accident, I-131 release could have occurred from a large amount of contaminated water in the basements of Units 2 and 3 reactor buildings because of the gas-liquid partition of I-131 and steam generation from the accumulated water by decay heat. The chemical form of certain fraction of released Cs could have been CsBO$$_{2}$$, which was formed by reaction of CsOH with the boron originated from the B$$_{4}$$C absorbers. The chemical form could affect not only the Cs-137 source term but also the environmental transport behavior. Te-129m release behavior showed that the release from the containment vessel could be affected by the difference in failure location between the top or middle height of drywell without pool and the bottom of suppression pool where the pool scrubbing is expected. These findings have never been considered in most of the existing severe accident codes such as MELCOR that have been developed based on the findings of the TMI-2 accident.

口頭

単一球形気泡からのエアロゾル除去のスケーリング則

茂木 孝介; 久木田 豊; 柴本 泰照

no journal, , 

プールスクラビングによるエアロゾル除去は、原子炉シビアアクシデント時に放射性物質の環境放出を抑制させる有力な手段のひとつとして、事故対策に適用されている。既存のスクラビングコードに採用されたモデルには、気泡内の粒子濃度分布を均一として扱うことで気泡内部の非定常な粒子運動の解析を省略し、粒子除去率を定常解として求めるという過度な単純化の課題がある。本項では気泡内気体流動場にHillの球形渦を用い、気体中を移行するエアロゾルをLagrangian粒子追跡することで、粒子数濃度分布を非定常で解析し除去率を求めた。その結果、気泡内を運動する低Stokes数の慣性粒子軌道に対してスケーリング則が成立することを明らかにした。これを用いて、単一粒子の軌道から気泡内の粒子不均一性を考慮した除染係数の計算方法を提案し、既存モデルと比較する。この様にして得られ除染係数にも同様なスケーリング則が成立することを示す。

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